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The modern differential geometry is a vast subject and while not specified exactly what you need the question is a bit too general. I would point out a few references.

It is resonable to look at :

another interesting thing by the same author :

Obviously you could find many helpful things here at the Wolfram Demonstrations :

For example :

Next it would be very helpful to look at this article in the Mathematica Journal by Murray Eisenberg and David J. M. Park, Jr. :

One should also look at the geometry section of

If you are looking for a package for tensor calculus, especially in General Relativity, the best choice is xAct made by José M. Martín-García (as far as I know he actually develops built-in functionality for the next version of Mathematica):

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